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Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

《环境科学与工程前沿（英文）》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0887-1

摘要： The distribution of NO - and VOC-sensitive regimes in the PRD are identified. The effectiveness of six popular chemical indicators for discriminating O sensitivity regimes is evaluated. Threshold levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO were derived and verified. The indicators H O /HNO and H O /NO performed best and maintained relatively stable threshold levels. Surface O production has a highly nonlinear relationship with its precursors. The spatial and temporal heterogeneity of O -NO -VOC-sensitivity regimes complicates the control- decision making. In this paper, the indicator method was used to establish the relationship between O sensitivity and assessment indicators. Six popular ratios indicating ozone-precursor sensitivity, HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO , were evaluated based on the distribution of NO - and VOC-sensitive regimes. WRF-Chem was used to study a serious ozone episode in fall over the Pearl River Delta (PRD). It was found that the south-west of the PRD is characterized by a VOC-sensitive regime, while its north-east is NO -sensitive, with a sharp transition area between the two regimes. All indicators produced good representations of the elevated ozone hours in the episode on 6 November 2009, with H O /HNO being the best indicator. The threshold sensitivity levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were estimated to be 0.41, 0.55, 10.2, 14.0, 19.1, and 0.38, respectively. Threshold intervals for the indicators H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were able to identify more than 95% of VOC- and NO -sensitive grids. The ozone episode on 16 November 16 2008 was used to independently verify the results, and it was found that only H O /HNO and H O /NO were able to differentiate the ozone sensitivity regime well. Hence, these two ratios are suggested as the most appropriate indicators for identifying fall ozone sensitivity in the PRD. Since the species used for indicators have seasonal variation, the utility of those indicators for other seasons should be investigated in the future work.

关键词： Ozone     Pearl River Delta (PRD)     Sensitivity regime     Photochemical indicator     Threshold levels    

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Investigation of bubble diameter and flow regime between water and dilute aqueous ethanol solutions in

Baharak SAJJADI, Mostafa Keshavarz MORAVEJI, Reza DAVARNEJAD

《化学科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 194-202 doi: 10.1007/s11705-010-1019-2

摘要： In this study, the effect of ethanol addition into pure water and its concentration on bubble diameter, gas hold-up and flow regimes were investigated in an airlift reactor. Air and water with ethanol (concentration ranging from 0%–1%, v/v) were as dispersed and continuous phases, respectively. Superficial gas velocity was considered as an effective parameter. Bubble size distribution was measured by photography and picture analysis at various concentrations of ethanol and various velocities of gas. Alcohol concentration enhancement caused bubble diameter to decrease. Furthermore, the bubbles diameter in pure water was nearly 4 times higher than that of ethanol with concentration of 1% (v/v) and also was 3.4 times higher than that of ethanol with concentration of 0.25% (v/v) at the highest aeration gas velocity inlet. For ethanol solutions in lower superficial gas velocity, a homogenous flow regime was observed. This trend continued to inlet gas velocity of about 0.4 cm/s. The transition flow regime occurred after this datum although in pure water, a homogenous flow regime was observed up to a superficial gas velocity of 0.7 cm/s. The gas hold-up in dilute ethanol solutions were more than (around 2 times) that of pure water and increased with increasing concentration of ethanol in those solutions.

关键词： airlift rector     bubble diameter     gas hold-up     flow regime     ethanol    

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Research on acoustic-structure sensitivity using FEM and BEM

ZHANG Jun, ZHAO Wenzhong, ZHANG Weiying

《机械工程前沿（英文）》 2007年 第2卷 第1期   页码 62-67 doi: 10.1007/s11465-007-0010-1

摘要： Acoustic-structure sensitivity is used to predict the change of acoustic pressure when a structure design variable is changed. The sensitivity is significant for reducing noise of structure. Using FEM (finite element method) and BEM (boundary element method) acoustic-structure sensitivity was formulated and presented. The dynamic response and response velocity sensitivity with respect to structure design variable were carried out by using structural FEM, the acoustic response and acoustic pressure sensitivity with respect to structure velocity were carried out by using acoustic BEM. Then, acoustic-structure sensitivity was computed by linking velocity sensitivity in FEM and acoustic sensitivity in BEM. This method was applied to an empty box as an example. Acoustic pressure sensitivity with respect to structure thickness achieved in frequency ranges 1 100 Hz, and its change rule along with stimulating frequency and design variable were analyzed. Results show that acoustic-structure sensitivity method linked with FEM and BEM is effective and correct.

关键词： sensitivity method     BEM     acoustic pressure     pressure sensitivity     frequency    

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Calculation of collision frequency function for aerosol particles in free molecule regime in presence

Xiaowei LUO, Yannick BENICHOU, Suyuan YU

《能源前沿（英文）》 2013年 第7卷 第4期   页码 506-510 doi: 10.1007/s11708-013-0275-5

摘要： The collision frequency function for aerosol particles has already been calculated for the free molecule regime and for the continuum range. The present work, taking into account the influence of internal force fields such as magnetic force, electric force and molecular forces, created by particles themselves, recalculated the collision frequency in the case of particles much smaller than the mean free path of the gas (free molecule regime). Attractive forces increase naturally the collision frequency, while repulsive forces decrease it. The calculation was performed for all types of central forces deriving from a potential, including Coulomb forces and Van der Waals forces.

关键词： aerosol particles     collision frequency function     coagulation    

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Kinetic roughening transition and missing regime transition of melt crystallized polybutene-1 tetragonal

Motoi YAMASHITA

《化学科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 125-134 doi: 10.1007/s11705-009-0001-3

摘要： The morphology and lateral growth rate of polybutene-1 ( -PB1) have been investigated for crystallization from the melt over a wide range of crystallization temperatures from 50 to 110°C. The morphology of -PB1 crystals is a rounded shape at crystallization temperatures lower than 85°C, while lamellar single crystals possess faceted morphology at higher crystallization temperatures. The kinetic roughening transition occurs around 85°C. The nucleation and growth mechanism for crystallization does not work below 85°C, since the growth face is rough. However, the growth rate shows the supercooling dependence derived from the nucleation and growth mechanism. The nucleation theory seems still to work even for rough surface growth. Possible mechanisms for the crystal growth of this polymer are discussed.

关键词： isotactic polybutene-1     tetragonal phase (form Ⅱ)     melt crystallization     growth rate     kinetic roughening     morphology    

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Parametric sensitivity analysis of cellular diaphragm wall

Xi CHEN, Wei XU

《结构与土木工程前沿（英文）》 2012年 第6卷 第4期   页码 358-364 doi: 10.1007/s11709-012-0177-3

摘要： The deformation law of the cellular diaphragm wall in deep foundation pits was studied through numerical simulation. Based on the example of the dock wall in engineering, the full three-dimensional finite element model was used to simulate the excavation of the foundation pit. Interaction between the cellular diaphragm wall and the soil was also taken into account in the calculation. The results indicated that the maximum lateral displacement, which is the evaluation index of sensitivity analysis, appeared on the top of the interior longitudinal wall with an excavation depth of 10 m. The centrifuge model test was carried out to study the deformation regulation for a cellular diaphragm wall. The most sensitive factor was found by adjusting the length of the partition wall, the spacing of the partition wall and the thickness of the wall. In the end, a suggestion was proposed to optimize the cellular diaphragm by adjusting the length of the partition wall.

关键词： cellular diaphragm wall     sensitivity analysis     optimization     centrifuge model test    

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Study of two-phase flow regime identification in horizontal tube bundles under vertical upward cross-flow

HUANG Xinghua, WANG Li, JIA Feng

《能源前沿（英文）》 2008年 第2卷 第3期   页码 333-338 doi: 10.1007/s11708-008-0043-0

摘要： A wavelet-transform based approach for flow regime identification in horizontal tube bundles under vertical upward cross-flow condition was presented. Tests on two-phase flow pattern of R134a were conducted under low mass velocity and flow boiling conditions over ranges of mass flux 4–25 kg/ms, vapor quality 0.02–0.90. Time series of differential pressure fluctuations were measured and analyzed with discrete wavelet transform. Different time-scale characteristics in bubbly flow, churn flow and annular flow were analyzed. The wavelet energy distributions over scales were found to be appropriate for flow regime identification. Based on the wavelet energy distribution over characteristic scales, a criterion of flow regime identification was proposed. The comparison with experiment results show that it is feasible to use the discrete wavelet transform as the tool of flow regime identification in horizontal tube bundles under vertical upward cross-flow condition.

关键词： two-phase     discrete     appropriate     wavelet-transform     criterion    

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Experimental study for the stratified to slug flow regime transition mechanism of gas-oil two-phase flow

LIU Yiping, YANG Weilin, WANG Jing

《能源前沿（英文）》 2008年 第2卷 第2期   页码 152-157 doi: 10.1007/s11708-008-0012-7

摘要： Theoretical relations that predict the transition from a stratified pattern to a slug pattern, including a one-dimensional wave model that contains less empiricism than the commonly used Taitel-Dukler model, and the ideal model for stratified flow for the gas-liquid flow in horizontal pipes are presented. Superficial velocities of each phase, as the onset of slugging occurs, were predicted, and theoretical analysis was conducted on the stratified to slug flow regime transition. The friction, existing between the fluid and pipe wall, and on the interface of two phases, was especially taken into account. A theoretical model was applied to an experiment about air-oil two-phase flow in a 50 mm horizontal pipe. The effect of pipe diameter on the transition was also studied. The results show that this approach gives a reasonable prediction over the whole range of flow rates, and better agreement has been achieved between predicted and measured critical parameters.

关键词： two-phase     Superficial     reasonable prediction     one-dimensional     gas-liquid    

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Probability strength design of steam turbine blade and sensitivity analysis with respect to random parameters

DUAN Wei

《能源前沿（英文）》 2008年 第2卷 第1期   页码 107-115 doi: 10.1007/s11708-008-0018-1

摘要： Many stochastic parameters have an effect on the reliability of a steam turbine blade during practical operation. To improve the reliability of blade design, it is necessary to take these stochastic parameters into account. An equal cross-section blade is investigated and a finite element model is built parametrically. Geometrical parameters, material parameters and load parameters of the blade are considered as input random variables while the maximum deflection and maximum equivalent stress are output random variables. Analysis file of the blade is compiled by deterministic finite element method and applied to be loop file to create sample points. A quadratic polynomial with cross terms is chosen to regress these samples by step-forward regression method and employed as a surrogate of numerical solver to drastically reduce the number of solvers call. Then, Monte Carlo method is used to obtain the statistical characteristics and cumulative distribution function of the maximum deflection and maximum equivalent stress of the blade. Probability sensitivity analysis, which combines the slope of the gradient and the width of the scatter range of the random input variables, is applied to evaluate how much the output parameters are influenced by the random input parameters. The scatter plots of structural responses with respect to the random input variables are illustrated to analyze how to change the input random variables to improve the reliability of the blade. The results show that combination of the finite element method, the response surface method and Monte Carlo method is an ideal way for the reliability analysis and probability strength design of the blade.

关键词： Probability sensitivity     sensitivity analysis     number     cross-section     statistical    

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Wheel tracking methods to evaluate moisture sensitivity of hot-mix asphalt mixtures

Jie HAN,Harihar Shiwakoti

《结构与土木工程前沿（英文）》 2016年 第10卷 第1期   页码 30-43 doi: 10.1007/s11709-016-0318-1

摘要： Existing test methods to determine moisture sensitivity in hot-mix asphalt (HMA) mixtures are time consuming and inconsistent. This research focused on wheel tracking devices to evaluate moisture sensitivity. The Asphalt Pavement Analyzer (APA) and the Hamburg Wheel Tracking Device (HWTD) were used for this research. Compacted cylindrical samples were fabricated using a Superpave Gyratory compactor. This study selected two most commonly used mixtures, SM-12.5A with PG 64-22 binder in overlay projects and SM-19A mixtures with PG 64-22 binder for major modification projects at Kansas Department of Transportation. Test results show that APA tests could induce stripping in most samples without any anti-stripping agent, which could be identified visually. However, APA results did not indicate any stripping inflection point while the HWTD results showed stripping inflection points, which are important to identify stripping potential of mixtures. The APA results show that wet tests are severe at lower temperatures. The HWTD results show improvement in the performance using anti-stripping agents at later stage. The HWTD test is more effective as a rapid test method in case of determining moisture sensitivity. Laboratory results from this study should be verified and correlated with field performance.

关键词： hot-mix asphalt     moisture sensitivity     rutting     wheel tracking test    

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Catalytic process modeling and sensitivity analysis of alkylation of benzene with ethanol over MIL-101

Ehsan Rahmani, Mohammad Rahmani

《化学科学与工程前沿（英文）》 2020年 第14卷 第6期   页码 1100-1111 doi: 10.1007/s11705-019-1891-3

摘要： A solvothermal method was used to synthesize MIL-101(Fe) and MIL-88(Fe), which were used for alkylation of benzene. The synthesized catalysts were characterized by X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscope, dynamic light scattering, and BET techniques. Metal-organic frameworks (MOFs) were modeled to investigate the catalytic performance and existence of mass transfer limitations. Calculated effectiveness factors revealed absence of internal and external mass transfer. Sensitivity analysis revealed best operating conditions over MIL-101 at 120°C and 5 bar and over MIL-88 at 142°C and 9 bar.

关键词： MOFs     alkylation     ethylbenzene     catalysts pellet model     kinetic model     sensitivity analysis    

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An antibiotic composite electrode for improving the sensitivity of electrochemically active biofilm biosensor

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1518-7

摘要：

• Antibiotic azithromycin employed in graphite electrode for EAB biosensor.

关键词： AZM@GP composite electrode     EAB-biosensor     Water quality early-warning    

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Global sensitivity analysis of certain and uncertain factors for a circular tunnel under seismic action

Nazim Abdul NARIMAN, Raja Rizwan HUSSAIN, Ilham Ibrahim MOHAMMAD, Peyman KARAMPOUR

《结构与土木工程前沿（英文）》 2019年 第13卷 第6期   页码 1289-1300 doi: 10.1007/s11709-019-0548-0

摘要： There are many certain and uncertain design factors which have unrevealed rational effects on the generation of tensile damage and the stability of the circular tunnels during seismic actions. In this research paper, we have dedicated three certain and four uncertain design factors to quantify their rational effects using numerical simulations and the Sobol’s sensitivity indices. Main effects and interaction effects between the design factors have been determined supporting on variance-based global sensitivity analysis. The results detected that the concrete modulus of elasticity for the tunnel lining has the greatest effect on the tensile damage generation in the tunnel lining during the seismic action. In the other direction, the interactions between the concrete density and both of concrete modulus of elasticity and tunnel diameter have appreciable effects on the tensile damage. Furthermore, the tunnel diameter has the deciding effect on the stability of the tunnel structure. While the interaction between the tunnel diameter and concrete density has appreciable effect on the stability process. It is worthy to mention that Sobol’s sensitivity indices manifested strong efficiency in detecting the roles of each design factor in cooperation with the numerical simulations explaining the responses of the circular tunnel during seismic actions.

关键词： shear waves     Sobol’s sensitivity indices     maximum principal stress     maximum overall displacement     tensile damage    

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Numerical study on natural convection in a square enclosure containing a rectangular heated cylinder

Jianhua LU, Zhaoli GUO, Zhenhua CHAI, Baochang SHI,

《能源前沿（英文）》 2009年 第3卷 第4期   页码 373-380 doi: 10.1007/s11708-009-0078-x

摘要： In this paper, the natural convection in a square enclosure with a rectangular heated cylinder is investigated via the lattice Boltzmann method. A detailed study is conducted on the effect of the cylinder width and the Rayleigh number on the fluid flow and heat transfer. The flow structures and heat transfer patterns are classified into eight buoyant regimes, i.e., four steady regimes, two periodic regimes, one multiple periodic regime, and one chaos regime, two of which are reported for the first time.

关键词： natural convection     buoyant regime     heated cylinder     lattice Boltzmann    

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photogeneration and extraction dynamics of polymer solar cells probed by a transient photocurrent nearby the regime

Boa Jin, Hyunmin Park, Yang Liu, Leijing Liu, Jongdeok An, Wenjing Tian, Chan Im

《化学科学与工程前沿（英文）》 2021年 第15卷 第1期   页码 164-179 doi: 10.1007/s11705-020-1976-z

摘要： To understand the complex behaviors of photogenerated charge carriers within polymer-based bulk-heterojunction-type solar cells, the charge-carrier photogeneration and extraction dynamics are simultaneously estimated using a transient photocurrent technique under various external-bias voltages, and a wide range of excitation intensities are analyzed. For this purpose, conventional devices with 80 nm thick active layers consisting of a blend of representative P3HT and PTB7 electron-donating polymers and proper electron-accepting fullerene derivatives were used. After the correction for the saturation behavior at a high excitation-intensity range nearby the regime of the space charge-limited current, the incident-photon-density-dependent maximum photocurrent densities at the initial peaks are discussed as the proportional measures of the charge-carrier-photogeneration facility. By comparing the total number of the extracted charge carriers to the total number of the incident photons and the number of the initially photogenerated charge carriers, the external quantum efficiencies as well as the extraction quantum efficiencies of the charge-carrier collection during a laser-pulse-induced transient photocurrent process were obtained. Subsequently, the charge-carrier concentration-dependent mobility values were obtained, and they are discussed in consideration of the additional influences of the charge-carrier losses from the device during the charge-carrier extraction that also affects the photocurrent-trace shape.

关键词： charge-carrier photogeneration     transient photocurrent     polymer solar cells     charge-carrier extraction     space charge-limited current    

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标题 作者 时间 类型 操作

Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

期刊论文

Investigation of bubble diameter and flow regime between water and dilute aqueous ethanol solutions in

Baharak SAJJADI, Mostafa Keshavarz MORAVEJI, Reza DAVARNEJAD

期刊论文

Research on acoustic-structure sensitivity using FEM and BEM

ZHANG Jun, ZHAO Wenzhong, ZHANG Weiying

期刊论文

Calculation of collision frequency function for aerosol particles in free molecule regime in presence

Xiaowei LUO, Yannick BENICHOU, Suyuan YU

期刊论文

Kinetic roughening transition and missing regime transition of melt crystallized polybutene-1 tetragonal

Motoi YAMASHITA

期刊论文

Parametric sensitivity analysis of cellular diaphragm wall

Xi CHEN, Wei XU

期刊论文

Study of two-phase flow regime identification in horizontal tube bundles under vertical upward cross-flow

HUANG Xinghua, WANG Li, JIA Feng

期刊论文

Experimental study for the stratified to slug flow regime transition mechanism of gas-oil two-phase flow

LIU Yiping, YANG Weilin, WANG Jing

期刊论文

Probability strength design of steam turbine blade and sensitivity analysis with respect to random parameters

DUAN Wei

期刊论文

Wheel tracking methods to evaluate moisture sensitivity of hot-mix asphalt mixtures

Jie HAN,Harihar Shiwakoti

期刊论文

Catalytic process modeling and sensitivity analysis of alkylation of benzene with ethanol over MIL-101

Ehsan Rahmani, Mohammad Rahmani

期刊论文

An antibiotic composite electrode for improving the sensitivity of electrochemically active biofilm biosensor

期刊论文

Global sensitivity analysis of certain and uncertain factors for a circular tunnel under seismic action

Nazim Abdul NARIMAN, Raja Rizwan HUSSAIN, Ilham Ibrahim MOHAMMAD, Peyman KARAMPOUR

期刊论文

Numerical study on natural convection in a square enclosure containing a rectangular heated cylinder

Jianhua LU, Zhaoli GUO, Zhenhua CHAI, Baochang SHI,

期刊论文

photogeneration and extraction dynamics of polymer solar cells probed by a transient photocurrent nearby the regime

Boa Jin, Hyunmin Park, Yang Liu, Leijing Liu, Jongdeok An, Wenjing Tian, Chan Im

期刊论文